Welcome to the forum
That can be a loaded question
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We'll actually need a bit more information to help.
The charge controller can be the main deciding factor for how the panels are conncted.
Is the charge controller a 12V , 24V or higher?
Since panels are 24V, my best guess would be that the controller is 24V as well.
IF you currently have the panels in parallel , which gives you 24Vdc with a possible 32A charging max, I would leave them alone. YOU could go with a MPPT controller and get a better charging rate, but they can be $$$$
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The other factor is the amount of current being used by ALL of the devices listed. Since you have 4 batteries , I would wire them up for 24Vdc which will give you 220A, then make sure your devices are not draining them down to less than 40% overnight or at a point where the sun can give back .
Hope that helps
Bruce S