This is a clever use of off-the-shelf parts that are cheap and easy to find. As you have stated, you are getting almost 500 gal/day (more than you needed) 100 ft above the source. Anyone can research the web and design an expensive and perfectly sized water wheel that has a very high efficiency, but regardless of any perceived inefficiencies, this did the job you wanted!
I don't want to sound as though I am picking at the design, but it is only pumping on the down stroke (actually, perfect for your particular application!), but half of the shafts rotation torque is unused. The other side of the wheel could use an identical pump to double the volume (180 degrees out of phase, of course). Also, because of the bell-shaped curve of feed-back resistance to pumping, I believe you could even put a third pump on the shaft without having to increase the diameter of the wheel or the width of the buckets (all three pumps phased at an even 120 degrees, like a Mercedes hood ornament).
I only point this out because by adding a second pump you can either increase the volume, or, by using smaller diameter pumps, you can keep the same volume but create a higher pressure in order to pump to a higher elevation.
You mention that you're making new buckets with stronger sheetmetal, what problem did you encounter with the thinner aluminum? Thanks for posting the pics.
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-Emo Phillips